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A Highly Stable Zeotype Mesoporous Zirconium Metal-Organic Framework with Ultralarge Pores
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för material- och miljökemi (MMK), Avdelningen för oorganisk kemi och strukturkemi.ORCID-id: 0000-0001-9800-3370
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2015 (engelsk)Inngår i: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 54, nr 1, s. 149-154Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

Through topological rationalization, a zeotype mesoporous Zr-containing metal-organic framework (MOF), namely PCN-777, has been designed and synthesized. PCN-777 exhibits the largest cage size of 3.8nm and the highest pore volume of 2.8cm(3)g(-1) among reported Zr-MOFs. Moreover, PCN-777 shows excellent stability in aqueous environments, which makes it an ideal candidate as a support to incorporate different functional moieties. Through facile internal surface modification, the interaction between PCN-777 and different guests can be varied to realize efficient immobilization.

sted, utgiver, år, opplag, sider
2015. Vol. 54, nr 1, s. 149-154
Emneord [en]
carboxylate ligands, host-guest systems, mesoporous materials, metal-organic frameworks, zirconium
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Identifikatorer
URN: urn:nbn:se:su:diva-113543DOI: 10.1002/anie.201409334ISI: 000347065100017OAI: oai:DiVA.org:su-113543DiVA, id: diva2:787082
Merknad

AuthorCount:10;

Tilgjengelig fra: 2015-02-09 Laget: 2015-02-04 Sist oppdatert: 2019-12-04bibliografisk kontrollert

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Su, JieZou, XiaodongZhou, Hong-Cai
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