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Versatile Heterogeneous Palladium Catalysts for Diverse Carbonylation Reactions under Atmospheric Carbon Monoxide Pressure
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för organisk kemi.
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för organisk kemi.ORCID-id: 0000-0002-2856-5295
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för organisk kemi.
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för material- och miljökemi (MMK).
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Rekke forfattare: 52018 (engelsk)Inngår i: ChemCatChem, ISSN 1867-3880, E-ISSN 1867-3899, Vol. 10, nr 5, s. 1089-1095Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

Herein, we report a versatile carbonylation protocol using heterogeneous Pd-0 nanoparticles supported on the metal-organic frameworks (MOFs) MIL-88B-NH2 (Fe/Cr). The synthesis of a vast array of carbonyls, which includes amides, esters, carboxylic acids, and -ketoamides, was achieved through mono- and dicarbonylation reactions. The selectivity could be controlled simply by tuning the reaction conditions. Superior activity and selectivity were recorded in some cases compared to that achieved with commercial Pd/C. However, the utility of an elaborate catalyst support is questionable and important reactivity and recyclability issues are discussed.

sted, utgiver, år, opplag, sider
2018. Vol. 10, nr 5, s. 1089-1095
Emneord [en]
carbonylation, heterogeneous catalysis, metal-organic frameworks, nanoparticles, palladium
HSV kategori
Identifikatorer
URN: urn:nbn:se:su:diva-154727DOI: 10.1002/cctc.201701439ISI: 000426844600030OAI: oai:DiVA.org:su-154727DiVA, id: diva2:1195015
Tilgjengelig fra: 2018-04-04 Laget: 2018-04-04 Sist oppdatert: 2019-12-12bibliografisk kontrollert

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