Ändra sökning
RefereraExporteraLänk till posten
Permanent länk

Direktlänk
Referera
Referensformat
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Annat format
Fler format
Språk
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Annat språk
Fler språk
Utmatningsformat
  • html
  • text
  • asciidoc
  • rtf
Observation-based estimates of the mass absorption cross-section of black and brown carbon and their contribution to aerosol light absorption in East Asia
Visa övriga samt affilieringar
Antal upphovsmän: 92019 (Engelska)Ingår i: Atmospheric Environment, ISSN 1352-2310, E-ISSN 1873-2844, Vol. 212, s. 65-74Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

In this study, we estimated the contribution of black carbon (BC) and brown carbon (BrC) to aerosol light absorption from surface in-situ and aerosol robotic network (AERONET) columnar observations. The mass absorption cross-section (MAC) of BC (MAC(BC)) was estimated to be 6.4 +/- 1.5 m(2) g(-1) at 565 mn from in-situ aerosol measurements at Gosan Climate Observatory (GCO), Korea, in January 2014, which was lower than those observed in polluted urban areas. A BrC MAC of 0.62 +/- 0.06 m(2) g(-1) (565 mn) in our estimate is approximately ten times lower than MACK at 565 nm. The contribution of BC and BrC to the carbonaceous aerosol absorption coefficient at 565 nm from the in-situ measurements was estimated at 88.1 +/- 7.4% and 11.9 +/- 7.4%, respectively at GCO. Similarly, the contribution of BC and BrC to the absorption aerosol optical depth (AAOD) for carbonaceous aerosol (CA), constrained by AERONET observations at 14 sites over East Asia by using different spectral dependences of the absorption (i.e., absorption Angstrom exponent) of BC and BrC, was 84.9 +/- 2.8% and 15.1 +/- 2.8% at 565 nm, respectively. The contribution of BC to CA AAOD was greater in urban sites than in the background areas, whereas the contribution of BrC to CA AAOD was higher in background sites. The overall contribution of BC to CA AAOD decreased by 73%-87% at 365 nm, and increased to 93%-97% at 860 nm. The contribution of BrC to CA AAOD decreased significantly with increasing wavelength from approximately 17% at 365 nm to 4% at 860 nm.

Ort, förlag, år, upplaga, sidor
2019. Vol. 212, s. 65-74
Nyckelord [en]
Black carbon, Brown carbon, Aerosol light absorption, Aerosol optical depth, Absorption aerosol optical depth, Mass absorption cross-section
Nationell ämneskategori
Geovetenskap och miljövetenskap
Identifikatorer
URN: urn:nbn:se:su:diva-170756DOI: 10.1016/j.atmosenv.2019.05.024ISI: 000474323500008OAI: oai:DiVA.org:su-170756DiVA, id: diva2:1338770
Tillgänglig från: 2019-07-24 Skapad: 2019-07-24 Senast uppdaterad: 2019-07-24Bibliografiskt granskad

Open Access i DiVA

Fulltext saknas i DiVA

Övriga länkar

Förlagets fulltext

Sök vidare i DiVA

Av författaren/redaktören
Gustafsson, ÖrjanAndersson, August
Av organisationen
Institutionen för miljövetenskap och analytisk kemi
I samma tidskrift
Atmospheric Environment
Geovetenskap och miljövetenskap

Sök vidare utanför DiVA

GoogleGoogle Scholar

doi
urn-nbn

Altmetricpoäng

doi
urn-nbn
Totalt: 17 träffar
RefereraExporteraLänk till posten
Permanent länk

Direktlänk
Referera
Referensformat
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Annat format
Fler format
Språk
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Annat språk
Fler språk
Utmatningsformat
  • html
  • text
  • asciidoc
  • rtf