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Ionic coherence in resonant above-threshold attosecond ionization spectroscopy
Stockholm University, Faculty of Science, Department of Physics.ORCID iD: 0000-0003-3444-1317
Number of Authors: 32023 (English)In: Physical Review A: covering atomic, molecular, and optical physics and quantum information, ISSN 2469-9926, E-ISSN 2469-9934, Vol. 107, no 3, article id 033103Article in journal (Refereed) Published
Abstract [en]

The ionization of atoms with sequences of attosecond pulses gives rise to excited ionic states that are entangled with the emitted photoelectron. Still, the ionic ensemble preserves some coherence that can be controlled through the laser parameters. In helium, control of the 2s/2p He+ coherence is mediated by the autoionizing states below the N=2 threshold [Phys. Rev. Res. 3, 023233 (2021)]. In the present work we study the role of the resonances both below and above the N=3 threshold on the coherence of the N=3 He+ ion, in the attosecond pump-probe ionization of the helium atom, which we simulate using the newstock ab initio code. Due to the fine-structure splitting of the N=3He+ level, the ionic dipole beats on a picosecond timescale. We show how, from the dipole beating, it is possible to reconstruct the polarization of the ion at its inception.

Place, publisher, year, edition, pages
2023. Vol. 107, no 3, article id 033103
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:su:diva-216914DOI: 10.1103/PhysRevA.107.033103ISI: 000952996500009Scopus ID: 2-s2.0-85149624075OAI: oai:DiVA.org:su-216914DiVA, id: diva2:1755371
Available from: 2023-05-08 Created: 2023-05-08 Last updated: 2023-05-08Bibliographically approved

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Lindroth, Eva

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