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Black carbon aerosols over Indian Ocean have unique source fingerprint and optical characteristics during monsoon season
Stockholm University, Faculty of Science, Department of Environmental Science. Stockholm University, Faculty of Science, The Bolin Centre for Climate Research (together with KTH & SMHI).ORCID iD: 0000-0002-4659-7055
Stockholm University, Faculty of Science, Department of Environmental Science. Stockholm University, Faculty of Science, The Bolin Centre for Climate Research (together with KTH & SMHI).ORCID iD: 0000-0002-5724-8256
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Number of Authors: 52023 (English)In: Proceedings of the National Academy of Sciences of the United States of America, ISSN 0027-8424, E-ISSN 1091-6490, Vol. 120, no 8, article id e2210005120Article in journal (Refereed) Published
Abstract [en]

Effects of aerosols such as black carbon (BC) on climate and buildup of the monsoon over the Indian Ocean are insufficiently quantified. Uncertain contributions from various natural and anthropogenic sources impede our understanding. Here, we use observations over 5 y of BC and its isotopes at a remote island observatory in northern Indian Ocean to constrain loadings and sources during little-studied monsoon season. Carbon-14 data show a highly variable yet largely fossil (65 ± 15%) source mixture. Combining carbon-14 with carbon-13 reveals the impact of African savanna burning, which occasionally approach 50% (48 ± 9%) of the total BC loadings. The BC mass-absorption cross-section for this regime is 7.6 ± 2.6 m2/g, with higher values during savanna fire input. Taken together, the combustion sources, longevity, and optical properties of BC aerosols over summertime Indian Ocean are different than the more-studied winter aerosol, with implications for chemical transport and climate model simulations of the Indian monsoon.

Place, publisher, year, edition, pages
2023. Vol. 120, no 8, article id e2210005120
Keywords [en]
air pollution, black carbon, long-range transport, Asian aerosol
National Category
Earth and Related Environmental Sciences
Identifiers
URN: urn:nbn:se:su:diva-217124DOI: 10.1073/pnas.2210005120ISI: 000964470200001PubMedID: 36780523Scopus ID: 2-s2.0-85148508743OAI: oai:DiVA.org:su-217124DiVA, id: diva2:1758114
Available from: 2023-05-22 Created: 2023-05-22 Last updated: 2025-02-07Bibliographically approved

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Andersson, AugustHolmstrand, HenryGustafsson, Örjan

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Department of Environmental ScienceThe Bolin Centre for Climate Research (together with KTH & SMHI)
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