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Terahertz ionic Kerr effect: Two-phonon contribution to the nonlinear optical response in insulators
Stockholm University, Faculty of Science, Department of Physics.ORCID iD: 0000-0001-8614-7991
Stockholm University, Faculty of Science, Department of Physics.ORCID iD: 0000-0002-6022-1206
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Number of Authors: 62024 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 109, no 2, article id 024309Article in journal (Refereed) Published
Abstract [en]

The THz Kerr effect measures the birefringence induced in an otherwise isotropic material by a strong THz pulse driving the Raman-active excitations of the systems. Here we provide experimental evidence of a sizable Kerr response in insulating SrTiO3 due to infrared-active lattice vibrations. Such a signal, named the ionic Kerr effect, is associated with the simultaneous excitation of multiple phonons. Thanks to a theoretical modeling of the time, polarization, and temperature dependence of the birefrengence, we can disentangle the ionic Kerr effect from the off-resonant electronic excitations, providing an alternative tunable mechanism to modulate the refractive index on ultrashort timescales via infrared active phonons.

Place, publisher, year, edition, pages
2024. Vol. 109, no 2, article id 024309
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Condensed Matter Physics
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URN: urn:nbn:se:su:diva-228961DOI: 10.1103/PhysRevB.109.024309ISI: 001173129900004Scopus ID: 2-s2.0-85182899370OAI: oai:DiVA.org:su-228961DiVA, id: diva2:1857632
Available from: 2024-05-14 Created: 2024-05-14 Last updated: 2024-05-14Bibliographically approved

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Basini, MartinaUnikandanunni, VivekBonetti, Stefano

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