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Multipolar multiferroics in 4d2/5d2 Mott insulators
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Number of Authors: 52025 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 111, no 20, article id L201107Article in journal (Refereed) Published
Abstract [en]

We extend the concept of conventional multiferroicity - where ferroelectric and ferromagnetic orders coexist - to include multipolar degrees of freedom. Specifically, we explore how this phenomenon emerges in 4d2/5d2 Mott insulators with strong spin-orbit and Hund's couplings. Our study uncovers the origin of magnetic multipolar interactions in these systems and demonstrates that a combination of quadrupolar and octupolar magnetic order can simultaneously induce both electrical quadrupolar moments and ferroelectric polarization. By expanding the multiferroic framework to higher-order multipoles, we reveal the possibility of coexisting multipolar orders of different or same ranks, paving the way for different functional properties in a large class of strongly correlated materials.

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2025. Vol. 111, no 20, article id L201107
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Condensed Matter Physics
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URN: urn:nbn:se:su:diva-244017DOI: 10.1103/PhysRevB.111.L201107ISI: 001494685200001Scopus ID: 2-s2.0-105005146417OAI: oai:DiVA.org:su-244017DiVA, id: diva2:1966596
Available from: 2025-06-10 Created: 2025-06-10 Last updated: 2025-06-10Bibliographically approved

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Balatsky, Alexander V.

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Nordic Institute for Theoretical Physics (Nordita)Department of Physics
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