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Volatility and Aging of Atmospheric Organic Aerosol
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för tillämpad miljövetenskap (ITM).
Vise andre og tillknytning
2014 (engelsk)Inngår i: Atmospheric and aerosol chemistry, Springer, 2014, s. 97-143Kapittel i bok, del av antologi (Fagfellevurdert)
Abstract [en]

Organic-aerosol phase partitioning (volatility) and oxidative aging are inextricably linked in the atmosphere because partitioning largely controls the rates and mechanisms of aging reactions as well as the actual amount of organic aerosol. Here we discuss those linkages, describing the basic theory of partitioning thermodynamics as well as the dynamics that may limit the approach to equilibrium under some conditions. We then discuss oxidative aging in three forms: homogeneous gas-phase oxidation, heterogeneous oxidation via uptake of gas-phase oxidants, and aqueous-phase oxidation. We present general scaling arguments to constrain the relative importance of these processes in the atmosphere, compared to each other and compared to the characteristic residence time of particles in the atmosphere.

sted, utgiver, år, opplag, sider
Springer, 2014. s. 97-143
Serie
Topics in Current Chemistry, ISSN 0340-1022 ; 339
Emneord [en]
Aerosols, Atmospheric Chemistry, Multiphase Chemistry
HSV kategori
Identifikatorer
URN: urn:nbn:se:su:diva-102491DOI: 10.1007/128_2012_355ISI: 000330882200004ISBN: 978-3-642-41215-8 (tryckt)ISBN: 978-3-642-41214-1 (tryckt)OAI: oai:DiVA.org:su-102491DiVA, id: diva2:710476
Merknad

AuthorCount:5;

Tilgjengelig fra: 2014-04-07 Laget: 2014-04-07 Sist oppdatert: 2014-04-07bibliografisk kontrollert

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