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Catchment-scale dissolved carbon concentrations and exportestimates across six subarctic streams in northern Sweden
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för naturgeografi.ORCID-id: 0000-0002-1137-648X
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för geologiska vetenskaper.
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2014 (Engelska)Ingår i: Biogeosciences, ISSN 1726-4170, E-ISSN 1726-4189, Vol. 11, s. 525-537Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

Climatic change is currently enhancing permafrostthawing and the flow of water through the landscape in subarcticand arctic catchments, with major consequences forthe carbon export to aquatic ecosystems. We studied streamwater carbon export in several tundra-dominated catchmentsin northern Sweden. There were clear seasonal differencesin both dissolved organic carbon (DOC) and dissolved inorganiccarbon (DIC) concentrations. The highest DOC concentrationsoccurred during the spring freshet while the highestDIC concentrations were always observed during winterbaseflow conditions for the six catchments considered in thisstudy. Long-term trends for the period 1982 to 2010 for oneof the streams showed that DIC concentrations has increasedby 9% during the 28 yr of measurement while no clear trendwas found for DOC. Similar increasing trends were alsofound for conductivity, Ca and Mg. When trends were discretizedinto individual months, we found a significant linearincrease in DIC concentrations with time for September,November and December. In these subarctic catchments, theannual mass of C exported as DIC was in the same orderof magnitude as DOC; the average proportion of DIC to thetotal dissolved C exported was 61% for the six streams. Furthermore,there was a direct relationship between total runoffand annual dissolved carbon fluxes for these six catchments.These relationships were more prevalent for annual DIC exportsthan annual DOC exports in this region. Our results alsohighlight that both DOC and DIC can be important in highlatitudeecosystems. This is particularly relevant in environmentswhere thawing permafrost and changes to subsurfaceice due to global warming can influence stream water fluxesof C. The large proportion of stream water DIC flux also hasimplications on regional C budgets and needs to be consideredin order to understand climate-induced feedback mechanismsacross the landscape.

Ort, förlag, år, upplaga, sidor
2014. Vol. 11, s. 525-537
Nationell ämneskategori
Geovetenskap och miljövetenskap
Forskningsämne
naturgeografi
Identifikatorer
URN: urn:nbn:se:su:diva-114282DOI: 10.5194/bg-11-525-2014OAI: oai:DiVA.org:su-114282DiVA, id: diva2:790680
Tillgänglig från: 2015-02-25 Skapad: 2015-02-25 Senast uppdaterad: 2019-12-09Bibliografiskt granskad
Ingår i avhandling
1. Waterborne Carbon in Northern Streams: Controls on dissolved carbon transport across sub-arctic Scandinavia
Öppna denna publikation i ny flik eller fönster >>Waterborne Carbon in Northern Streams: Controls on dissolved carbon transport across sub-arctic Scandinavia
2015 (Engelska)Doktorsavhandling, sammanläggning (Övrigt vetenskapligt)
Abstract [en]

Waterborne carbon (C) forms an active and significant part of the global C cycle, which is important in theArctic where greater temperature increases and variability are anticipated relative to the rest of the globe withpotential implications for the C cycle. Understanding and quantification of the current processes governing themovement of C by connecting terrestrial and marine systems is necessary to better estimate future changes ofwaterborne C. This thesis investigates how the sub-arctic landscape influences the waterborne carbon exportby combining data-driven and modeling methods across spatial and temporal scales. First, a study of the stateof total organic carbon monitoring in northern Scandinavia was carried out using national-scale monitoringdata and detailed data from scientific literature. This study, which highlights the consistency in land cover andhydroclimatic controls on waterborne C across northern Scandinavia, was combined with three more detailedstudies leveraging field measurements and modeling. These focused on the Abisko region to provide insightto processes and mechanisms across scales. The thesis highlights that the governing transport mechanismsof dissolved organic and inorganic carbon (DOC and DIC respectively) are fundamentally different due todifferences in release rates associated with the nature of their terrestrial sources (geogenic and organic matterrespectively). As such, the DIC mass flux exhibits a high flow-dependence whereas DOC is relatively flowindependent.Furthermore, these investigations identified significant relationships between waterborne C andbiogeophysical as well as hydroclimatic variables across large to small spatial scales. This thesis demonstratesthat both surface and sub-surface hydrological processes (such as flow pathway distributions) in combinationwith distributions of C sources and associated release rates are prerequisite for understanding waterborne Cdynamics in northern streams.

Ort, förlag, år, upplaga, sidor
Stockholm: Department of Physical Geography, Stockholms Universitet, 2015
Serie
Dissertations from the Department of Physical Geography, ISSN 1653-7211 ; 48
Nyckelord
dissolved carbon, DOC, DIC, TOC, sub-arctic, hydrology, Abisko
Nationell ämneskategori
Naturgeografi
Forskningsämne
naturgeografi
Identifikatorer
urn:nbn:se:su:diva-115883 (URN)978-91-7649-141-6 (ISBN)
Disputation
2015-05-22, Nordenskiöldsalen, Geovetenskapens hus, Svante Arrhenius väg 12, Stockholm, 13:00 (Engelska)
Opponent
Handledare
Forskningsfinansiär
Vetenskapsrådet, 2007-8393
Anmärkning

At the time of the doctoral defense, the following papers were unpublished and had a status as follows: Paper 1: Submitted. Paper 4: Accepted.

Tillgänglig från: 2015-04-29 Skapad: 2015-04-07 Senast uppdaterad: 2020-01-17Bibliografiskt granskad

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Av författaren/redaktören
Lyon, Steve W.Mörth, Carl-MagnusJantze, Elin J.Destouni, GeorgiaHumborg, Christoph
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Institutionen för naturgeografiInstitutionen för geologiska vetenskaperInstitutionen för tillämpad miljövetenskap (ITM)
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