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Direct and Stereospecific [3+2] Synthesis of Pyrrolidines from Simple Unactivated Alkenes
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
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Number of Authors: 5
2017 (English)In: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 56, no 42, 12962-12966 p.Article in journal (Refereed) Published
Abstract [en]

Pyrrolidines are important heterocyclic compounds with endless applications in organic synthesis, metal catalysis, and organocatalysis. Their potential as ligands for first-row transition-metal catalysts inspired a new method to access complex poly-heterocyclic pyrrolidines in one step from available materials. This fundamental step forward is based on the discovery of an essential organoaluminum promoter that engages unactivated and electron-rich olefins in intermolecular [3+2] cycloadditions.

Place, publisher, year, edition, pages
2017. Vol. 56, no 42, 12962-12966 p.
Keyword [en]
alkenes, aluminum, C-C coupling, cycloaddition, nitrogen heterocycles
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-147842DOI: 10.1002/anie.201706682ISI: 000412189700028PubMedID: 28816407OAI: oai:DiVA.org:su-147842DiVA: diva2:1153977
Available from: 2017-11-01 Created: 2017-11-01 Last updated: 2017-11-01Bibliographically approved

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Montesinos-Magraner, MarcMendoza, Abraham
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