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Regioselective Iridium-Catalyzed Asymmetric Monohydrogenation of 1,4-Dienes
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
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Number of Authors: 7
2017 (English)In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126, Vol. 139, no 41, 14470-14475 p.Article in journal (Refereed) Published
Abstract [en]

A highly efficient regio- and enantioselective monohydrogenation of 1,4-dienes has been realized using an iridium catalyst with a chiral N,P-ligand under mild conditions. The substrate scope was studied and included both unfunctionalized as well as functionalized substituents on the meta- or para-position. Substrates having substituents with functionalities such as silyl protected alcohols or ketals were monohydrogenated in high regioselectivity and high enantiomeric excess (up to 98% ee).

Place, publisher, year, edition, pages
2017. Vol. 139, no 41, 14470-14475 p.
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Organic Chemistry
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URN: urn:nbn:se:su:diva-149001DOI: 10.1021/jacs.7b06829ISI: 000413503300025PubMedID: 28930455OAI: oai:DiVA.org:su-149001DiVA: diva2:1160385
Available from: 2017-11-27 Created: 2017-11-27 Last updated: 2017-11-27Bibliographically approved

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