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Embedded Isoreticular Zeolites: Concept and Beyond
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
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Number of Authors: 62017 (English)In: Chemistry - A European Journal, ISSN 0947-6539, E-ISSN 1521-3765, Vol. 23, no 63, p. 15922-15929Article in journal (Refereed) Published
Abstract [en]

The structure solution, prediction, and targeted synthesis of a family of embedded isoreticular zeolites (EIZs) with expanding structural complexity, denoted the RHO family, were reported recently. Here, the naming and building rules of body-centered cubic EIZs with the lta cage as the lattice point are presented. The rearrangement of a pair of pau and d8r cages between two lta cages and its repetitive insertion, combined with the strong reflections and fragment methods, allows the creation of three other new zeolite families, designated the HPO, RHO(b), and KFI families. Among them, the KFI family is found to be the only EIZ family, on the basis of the similarity of structure factor amplitudes and phases of strong reflections, that is, structural coding, within its family members. The structural credibility of this family is confirmed by both local interatomic distances and T-T-T angle analyses. The existence of tetragonal EIZ families is also demonstrated. The overall results provide useful insights into the prediction of unprecedented EIZ families.

Place, publisher, year, edition, pages
2017. Vol. 23, no 63, p. 15922-15929
Keywords [en]
crystal engineering, embedded isoreticular zeolites, microporous materials, naming rules, structure prediction, zeolites
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:su:diva-149809DOI: 10.1002/chem.201702417ISI: 000414990400015PubMedID: 28786145OAI: oai:DiVA.org:su-149809DiVA, id: diva2:1167357
Available from: 2017-12-18 Created: 2017-12-18 Last updated: 2017-12-18Bibliographically approved

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