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Probing the OH Stretch in Different Local Environments in Liquid Water
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Number of Authors: 6
2017 (English)In: Journal of Physical Chemistry Letters, ISSN 1948-7185, E-ISSN 1948-7185, Vol. 8, no 22, 5487-5491 p.Article in journal (Refereed) Published
Abstract [en]

We use resonant inelastic X-ray scattering (RIXS) to resolve vibrational losses corresponding to the OH stretch where the X-ray absorption process allows us to selectively probe different structural subensembles in liquid water. The results point to a unified interpretation of X-ray and vibrational spectroscopic data in line with a picture of two classes of structural environments in the liquid at ambient conditions with predominantly close-packed high-density liquid (HDL) and occasional local fluctuations into strongly tetrahedral low-density liquid (LDL).

Place, publisher, year, edition, pages
2017. Vol. 8, no 22, 5487-5491 p.
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Chemical Sciences Nano Technology Materials Engineering Physical Sciences
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URN: urn:nbn:se:su:diva-149799DOI: 10.1021/acs.jpclett.7b02060ISI: 000416291600004PubMedID: 29108417OAI: oai:DiVA.org:su-149799DiVA: diva2:1167758
Available from: 2017-12-19 Created: 2017-12-19 Last updated: 2017-12-19Bibliographically approved

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Pettersson, Lars G. M.Nilsson, Anders
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