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Design and synthesis of biobased epoxy thermosets from biorenewable resources
Stockholm University, Faculty of Science, Department of Organic Chemistry.
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Number of Authors: 122017 (English)In: Comptes rendus. Chimie, ISSN 1631-0748, E-ISSN 1878-1543, Vol. 20, no 11-12, p. 1006-1016Article in journal (Refereed) Published
Abstract [en]

Biobased diepoxy synthons derived from isoeugenol, eugenol or resorcinol (DGE-isoEu, DGE-Eu and DGER, respectively) have been used as epoxy monomers in replacement of the diglycidyl ether of bisphenol A (DGEBA). Their curing with six different biobased anhydride hardeners leads to fully biobased epoxy thermosets. These materials exhibit interesting thermal and mechanical properties comparable to those obtained with conventional petrosourced DGEBA-based epoxy resins cured in similar conditions. In particular, a high T-g in the range of 90-130 degrees C and instantaneous moduli higher than 4.3 GPa have been recorded. These good performances are very encouraging, making these new fully biobased epoxy thermosets compatible with the usual structural application of epoxy materials.

Place, publisher, year, edition, pages
2017. Vol. 20, no 11-12, p. 1006-1016
Keywords [en]
Biobased resins, DEGBA alternative, Epoxy-anhydride thermosets, Curing process, Nanoindentation
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-152656DOI: 10.1016/j.crci.2017.10.005ISI: 000418629300004OAI: oai:DiVA.org:su-152656DiVA, id: diva2:1182191
Available from: 2018-02-12 Created: 2018-02-12 Last updated: 2018-02-12Bibliographically approved

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