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Highly Diastereo- and Enantioselective Cascade Synthesis of Bicyclic Lactams in One-Pot
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
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Number of Authors: 62018 (English)In: European Journal of Organic Chemistry, ISSN 1434-193X, E-ISSN 1099-0690, no 9, p. 1158-1164Article in journal (Refereed) Published
Abstract [en]

A versatile and highly stereoselective synthetic route to functionalized bi- and tricyclic lactams (up to > 20:1 dr and 99% ee) in one pot from simple starting materials (allylic alcohols, enals, diamines and amino alcohols) using cascade transformations promoted by chiral amine/BrOnsted or metal/chiral amine/BrOnsted relay catalysis is disclosed. Here molecular oxygen is employed as the terminal oxidant for the latter relay catalysis approach.

Place, publisher, year, edition, pages
2018. no 9, p. 1158-1164
Keywords [en]
Relay catalysis, Asymmetric catalysis, Bicyclic lactams, Hemiaminal ether, Aminal
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:su:diva-154776DOI: 10.1002/ejoc.201701789ISI: 000426771400009OAI: oai:DiVA.org:su-154776DiVA, id: diva2:1198692
Available from: 2018-04-18 Created: 2018-04-18 Last updated: 2018-04-18Bibliographically approved

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Sun, Junliang
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