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Attosecond transient absorption spectrum of argon at the L-2,L-3 edge
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Number of Authors: 10
2018 (English)In: Physical Review A: covering atomic, molecular, and optical physics and quantum information, ISSN 2469-9926, E-ISSN 2469-9934, Vol. 97, no 3, article id 031407Article in journal (Refereed) Published
Abstract [en]

Progress in high-harmonic generation has led to high-energy attosecond pulses with cutoff above the carbon 1s edge (283.8 eV). These pulses are essential to extend time-resolved spectroscopies to the water window in order to control electron dynamics in solvated organic species. Here we report a step towards this goal: the measurement, with subcycle time resolution, of the attosecond transient absorption spectrum of argon at the 2p(-1) L-2,L-3 edge (similar to 250 eV) in the presence of a short-wave infrared control pulse. The measurements, supported by theoretical simulations, demonstrate the concurrent role of Auger decay and tunnel ionization in the driven evolution of inner-valence holes of polyelectronic atoms.

Place, publisher, year, edition, pages
2018. Vol. 97, no 3, article id 031407
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Physical Sciences
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URN: urn:nbn:se:su:diva-156050DOI: 10.1103/PhysRevA.97.031407ISI: 000428774000001OAI: oai:DiVA.org:su-156050DiVA, id: diva2:1202958
Available from: 2018-05-02 Created: 2018-05-02 Last updated: 2018-05-02Bibliographically approved

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