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Diastereoselective Synthesis of Polycyclic Indolizines with 2-(2-Enynyl)pyridines and Enamines
Stockholm University, Faculty of Science, Department of Organic Chemistry.ORCID iD: 0000-0002-6536-8506
Stockholm University, Faculty of Science, Department of Organic Chemistry.ORCID iD: 0000-0002-9085-0476
Stockholm University, Faculty of Science, Department of Organic Chemistry.ORCID iD: 0000-0002-9085-0476
Number of Authors: 32018 (English)In: Organic Letters, ISSN 1523-7060, E-ISSN 1523-7052, Vol. 20, no 12, p. 3691-3694Article in journal (Refereed) Published
Abstract [en]

A diastereoselective metal-catalyzed reaction of 2-(2-enynyl)pyridines and cyclic enamines is reported. The method provides access to a variety of substituted indolizine derivatives by variation of the enyne component and the reaction conditions. Performing the reaction using a preformed enamine led to the formation of polycyclic indolizines. With in situ generated enamines, ketone-containing indolizine derivatives were obtained. An asymmetric reaction of 2-(2-enynyl)pyridines and enamines generated from an aldehyde and a catalytic amount of amine is presented.

Place, publisher, year, edition, pages
2018. Vol. 20, no 12, p. 3691-3694
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-158259DOI: 10.1021/acs.orglett.8b01498ISI: 000435746500059PubMedID: 29878789OAI: oai:DiVA.org:su-158259DiVA, id: diva2:1237597
Available from: 2018-08-09 Created: 2018-08-09 Last updated: 2018-08-09Bibliographically approved

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Pathipati, Stalin R.van der Werf, AngelaSelander, Nicklas
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