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Resonant inelastic x-ray incarnation of Young's double-slit experiment
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Number of Authors: 152019 (English)In: Science Advances, E-ISSN 2375-2548, Vol. 5, no 1, article id eaav4020Article in journal (Refereed) Published
Abstract [en]

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: The elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation of Young's experiment and demonstrate that resonant inelastic x-ray scattering (RIXS) measures interference patterns, which reveal the symmetry and character of electronic excited states in the same way as elastic scattering does for the ground state. A prototypical example is provided by the quasi-molecular electronic structure of insulating Ba3CeIr2O9 with structural Ir dimers and strong spin-orbit coupling. The double slits in this resonant experiment are the highly localized core levels of the two Ir atoms within a dimer. The clear double-slit-type sinusoidal interference patterns that we observe allow us to characterize the electronic excitations, demonstrating the power of RIXS interferometry to unravel the electronic structure of solids containing, e.g., dimers, trimers, ladders, or other superstructures.

Place, publisher, year, edition, pages
2019. Vol. 5, no 1, article id eaav4020
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Physical Sciences
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URN: urn:nbn:se:su:diva-166622DOI: 10.1126/sciadv.aav4020ISI: 000457547900042PubMedID: 30746479OAI: oai:DiVA.org:su-166622DiVA, id: diva2:1297569
Available from: 2019-03-20 Created: 2019-03-20 Last updated: 2019-03-20Bibliographically approved

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Hermanns, Maria
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Department of PhysicsNordic Institute for Theoretical Physics (Nordita)
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