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Storage time dependent photodissociation action spectroscopy of polycyclic aromatic hydrocarbon cations in the cryogenic electrostatic storage ring DESIREE
Stockholm University, Faculty of Science, Department of Physics.
Stockholm University, Faculty of Science, Department of Physics.
Stockholm University, Faculty of Science, Department of Physics.
Stockholm University, Faculty of Science, Department of Physics.
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Number of Authors: 52019 (English)In: Faraday discussions (Online), ISSN 1359-6640, E-ISSN 1364-5498, Vol. 217, p. 126-137Article in journal (Refereed) Published
Abstract [en]

The multi-photon photodissociation action spectrum of the coronene cation (C24H12+) has been measured in the cryogenic electrostatic storage ring DESIREE (Double ElectroStatic Ion Ring ExpEriment) as a function of storage time. These measurements reveal not only the intrinsic absorption profile of isolated coronene cations, but also the rate at which hot-band absorptions are quenched by radiative cooling. Just after injection, the action spectrum is severely reddened by hot-band absorptions. These hot bands fade with a time constant of 200 ms, which is consistent with radiative cooling via infrared emission from vibrational transitions. A comparison of the present results to those obtained in cryogenic ion trap experiments is discussed at length.

Place, publisher, year, edition, pages
2019. Vol. 217, p. 126-137
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Physical Sciences
Identifiers
URN: urn:nbn:se:su:diva-171783DOI: 10.1039/c8fd00161hISI: 000476809000007PubMedID: 31012449OAI: oai:DiVA.org:su-171783DiVA, id: diva2:1346187
Available from: 2019-08-27 Created: 2019-08-27 Last updated: 2019-08-27Bibliographically approved

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Stockett, Mark H.Björkhage, MikaelCederquist, HenrikSchmidt, Henning T.Zettergren, Henning
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