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Multiplicity conversion based on intramolecular triplet-to-singlet energy transfer
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
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Number of Authors: 72019 (English)In: Science Advances, E-ISSN 2375-2548, Vol. 5, no 9, article id eaaw5978Article in journal (Refereed) Published
Abstract [en]

The ability to convert between molecular spin states is of utmost importance in materials chemistry. Forster-type energy transfer is based on dipole-dipole interactions and can therefore theoretically be used to convert between molecular spin states. Here, a molecular dyad that is capable of transferring energy from an excited triplet state to an excited singlet state is presented. The rate of conversion between these states was shown to be 36 times faster than the rate of emission from the isolated triplet state. This dyad provides the first solid proof that Forster-type triplet-to-singlet energy transfer is possible, revealing a method to increase the rate of light extraction from excited triplet states.

Place, publisher, year, edition, pages
2019. Vol. 5, no 9, article id eaaw5978
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Chemical Sciences
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URN: urn:nbn:se:su:diva-175725DOI: 10.1126/sciadv.aaw5978ISI: 000491128800061PubMedID: 31555728OAI: oai:DiVA.org:su-175725DiVA, id: diva2:1369193
Available from: 2019-11-11 Created: 2019-11-11 Last updated: 2019-11-11Bibliographically approved

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Hertzog, M.Iqbal, Muhammad NaeemEriksson, LarsBorjesson, K.
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