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CO Chemisorption on Vicinal Rh(111) Surfaces Studied with a Curved Crystal
Stockholm University, Faculty of Science, Department of Physics. Lund University, Sweden.
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Number of Authors: 82020 (English)In: The Journal of Physical Chemistry C, ISSN 1932-7447, E-ISSN 1932-7455, Vol. 124, no 17, p. 9305-9313Article in journal (Refereed) Published
Abstract [en]

Curved crystal surfaces enable the systematic and accurate comparison of physical and chemical processes for a full set of vicinal crystal planes, which are probed in the very same environment. Here, we examine the early stages of the CO chemisorption on vicinal Rh(111) surfaces using a curved Rh crystal that exposes a smoothly variable density of {100} (A-type) and {111} (B-type) steps. We readily identify and quanti step and terrace species by resolving their respective core-level lines using X-ray photoelectron spectroscopy at different locations on the curved surface. Uptake experiments show similar sticking probabilities at all surface planes, subtle asymmetries between A- and B-type steps, and significantly lower saturation coverage at densely stepped surfaces as compared to the (111) plane. The analysis of the C is intensity variation across the curved sample allows us to discuss the adsorption geometry around the step edge.

Place, publisher, year, edition, pages
2020. Vol. 124, no 17, p. 9305-9313
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Physical Sciences
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URN: urn:nbn:se:su:diva-181968DOI: 10.1021/acs.jpcc.0c00039ISI: 000529873300024Scopus ID: 2-s2.0-85084812711OAI: oai:DiVA.org:su-181968DiVA, id: diva2:1438119
Available from: 2020-06-10 Created: 2020-06-10 Last updated: 2022-11-07Bibliographically approved

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Shipilin, Mikhail

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