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Isotope constraints of the strong influence of biomass burning to climate-forcing Black Carbon aerosols over Southeast Asia
Stockholm University, Faculty of Science, Department of Environmental Science. Jinan University, China; Chinese Academy of Sciences, China.
Stockholm University, Faculty of Science, Department of Environmental Science.
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Number of Authors: 132020 (English)In: Science of the Total Environment, ISSN 0048-9697, E-ISSN 1879-1026, Vol. 744, article id 140359Article in journal (Refereed) Published
Abstract [en]

Black Carbon (BC) deteriorates air quality and contributes to climate warming, yet its regionally- and seasonally-varying emission sources are poorly constrained. Here we employ natural abundance radiocarbon (C-14) measurements of BC intercepted at a northern Malaysia regional receptor site, Bachok, to quantify the relative biomass vs. fossil source contributions of atmospheric BC, in a first year-round study for SE Asia (December 2015-December 2016). The annual average C-14 signature suggests as large contributions from biomass burning as from fossil fuel combustion. This is similar to findings from analogous measurements at S Asian receptors sites (similar to 50% biomass burning), while E Asia sites are dominated by fossil emission (similar to 20% biomass burning). The C-14-based source fingerprinting of BC in the dry spring season in SE Asia signals an even more elevated biomass burning contribution (similar to 70% or even higher), presumably from forest, shrub and agricultural fires. This is consistent with this period showing also elevated ratio of organic carbon to BC (up from similar to 5 to 30) and estimates of BC emissions from satellite fire data. Hence, the present study emphasizes the importance of mitigating dry season vegetation fires in SE Asia.

Place, publisher, year, edition, pages
2020. Vol. 744, article id 140359
Keywords [en]
Black Carbon, Radiocarbon, Biomass burning, SE Asia
National Category
Earth and Related Environmental Sciences
Identifiers
URN: urn:nbn:se:su:diva-187496DOI: 10.1016/j.scitotenv.2020.140359ISI: 000578951100001PubMedID: 32688001OAI: oai:DiVA.org:su-187496DiVA, id: diva2:1509728
Available from: 2020-12-14 Created: 2020-12-14 Last updated: 2025-02-07Bibliographically approved

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Andersson, AugustCheng, ZhinengGustafsson, Örjan

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