Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Fluorinated Cationic Iridium(III) Complex Yielding an Exceptional, Efficient, and Long-Lived Red-Light-Emitting Electrochemical Cell
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).ORCID iD: 0000-0002-2743-8550
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).ORCID iD: 0000-0002-0265-7431
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).ORCID iD: 0000-0003-0763-1457
Show others and affiliations
Number of Authors: 62020 (English)In: ACS Applied Energy Materials, E-ISSN 2574-0962, Vol. 3, no 9, p. 9271-9277Article in journal (Refereed) Published
Abstract [en]

A carefully designed red-light-emitting iridium (III) cationic complex yields light-emitting electrochemical cells (LECs) with exceptional efficiency and stability [Ir(4Fppy)(2)(biq)][PF6] (4Fppy = 2-(4-fluorophenyl)pyridinato, biq = 2,2'-biquinoline), whose structure was authenticated by single-crystal X-ray diffraction, emits in the red region of light with photoluminescence (upon 360 nm excitation) and electroluminescence maxima at 629 nm. Astonishingly, it is based on a fluorinated ligand, a design concept more commonly used for green emitter materials. Pairing it with a ligand that has comparatively low-lying frontier orbitals allows for a red shift of the band gap. The uncommon electronic structure of the complex allows overcoming the common problem of strong metal-ligand antibonding interactions in the excited state, rendering it extremely stable under operation. The complex displays a high photoluminescence quantum yield of 27.1% giving rise to an extremely efficient LEC with an initial maximum luminance of 326 cd m(-2), current efficiency of 3.26 cd A(-1), and power efficiency of 2.27 Im W-1, surpassing the current state of the art. Remarkably, the efficient red LEC has a lifetime of 167 h when driven under a block-wave pulsed current at a frequency of 1000 Hz, an average current density of 100 A m(-2), and a duty cycle of 50%. Increasing the duty cycle to 75% led to a decrease in the device average voltage, increasing the power efficiency to an exceptional value of 2.97 Im W-1 without compromising the device stability.

Place, publisher, year, edition, pages
2020. Vol. 3, no 9, p. 9271-9277
Keywords [en]
electroluminescence, Ir complexes, light-emitting electrochemical cells, lighting, organic lighting
National Category
Chemical Sciences Physical Sciences
Identifiers
URN: urn:nbn:se:su:diva-187698DOI: 10.1021/acsaem.0c01600ISI: 000576676900123OAI: oai:DiVA.org:su-187698DiVA, id: diva2:1511135
Available from: 2020-12-17 Created: 2020-12-17 Last updated: 2022-02-25Bibliographically approved

Open Access in DiVA

No full text in DiVA

Other links

Publisher's full text

Authority records

Pei, HanwenBousrez, GuillaumeSmetana, VolodymyrMudring, Anja-Verena

Search in DiVA

By author/editor
Pei, HanwenBousrez, GuillaumeSmetana, VolodymyrMudring, Anja-Verena
By organisation
Department of Materials and Environmental Chemistry (MMK)
In the same journal
ACS Applied Energy Materials
Chemical SciencesPhysical Sciences

Search outside of DiVA

GoogleGoogle Scholar

doi
urn-nbn

Altmetric score

doi
urn-nbn
Total: 51 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf