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High Thermopower in a Zn-Based 3D Semiconductive Metal-Organic Framework
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).ORCID iD: 0000-0002-4575-7870
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Number of Authors: 72020 (English)In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126, Vol. 142, no 49, p. 20531-20535Article in journal (Refereed) Published
Abstract [en]

Conductive metal-organic frameworks (c-MOFs) have drawn increasing attention for their outstanding performance in energy-related applications. However, the majority of reported c-MOFs are based on 2D structures. Synthetic strategies for 3D c-MOFs are under-explored, leaving unrealized functionality in both their structures and properties. Herein we report Zn-HAB, a 3D c-MOF comprised of hexaaminobenzene and Zn(II). Zn-HAB is shown to have microporosity with a band gap of approximately 1.68 eV, resulting in a moderate conductivity of 0.86 mS cm(-1) and a high Seebeck coefficient of 200 mu V K-1 at 300 K. The power factor of 3.44 nW m(-1) K-2 constitutes the first report of the thermoelectric properties of an intrinsically conductive 3D MOF.

Place, publisher, year, edition, pages
2020. Vol. 142, no 49, p. 20531-20535
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Chemical Sciences
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URN: urn:nbn:se:su:diva-190668DOI: 10.1021/jacs.0c09573ISI: 000599506900005PubMedID: 33226798OAI: oai:DiVA.org:su-190668DiVA, id: diva2:1533014
Available from: 2021-03-03 Created: 2021-03-03 Last updated: 2022-02-25Bibliographically approved

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Park, JihyeHinckley, Allison C.Huang, ZhehaoChen, GanZou, XiaodongBao, Zhenan

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