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Molecular strain in the active/deactive-transition modulates domain coupling in respiratory complex I
Stockholm University, Faculty of Science, Department of Biochemistry and Biophysics.
Stockholm University, Faculty of Science, Department of Biochemistry and Biophysics.ORCID iD: 0000-0003-4464-6324
Number of Authors: 22021 (English)In: Biochimica et Biophysica Acta - Bioenergetics, ISSN 0005-2728, E-ISSN 1879-2650, Vol. 1862, no 5, article id 148382Article in journal (Refereed) Published
Abstract [en]

Complex I functions as a primary redox-driven proton pump in aerobic respiratory chains, establishing a proton motive force that powers ATP synthesis and active transport. Recent cryo-electron microscopy (cryo-EM) experiments have resolved the mammalian complex I in the biomedically relevant active (A) and deactive (D) states (Zhu et al., 2016; Fiedorczuk et al., 2016; Agip et al., 2018 [1-3]) that could regulate enzyme turnover, but it still remains unclear how the conformational state and activity are linked. We show here how global motion along the A/D transition accumulates molecular strain at specific coupling regions important for both redox chemistry and proton pumping. Our data suggest that the A/D motion modulates force propagation pathways between the substrate-binding site and the proton pumping machinery that could alter electrostatic and conformational coupling across large distances. Our findings provide a molecular basis to understand how global protein dynamics can modulate the biological activity of large molecular complexes.

Place, publisher, year, edition, pages
2021. Vol. 1862, no 5, article id 148382
Keywords [en]
Bioenergetics, NADH:ubiquinone oxidoreductase, Network models, Active/deactive transition, Molecular strain
National Category
Biological Sciences
Identifiers
URN: urn:nbn:se:su:diva-193027DOI: 10.1016/j.bbabio.2021.148382ISI: 000636042900003PubMedID: 33513365OAI: oai:DiVA.org:su-193027DiVA, id: diva2:1554021
Available from: 2021-05-11 Created: 2021-05-11 Last updated: 2022-02-25Bibliographically approved

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Di Luca, AndreaKaila, Ville R.

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