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Implementation and validation of the relativistic transient absorption theory within the dipole approximation
Stockholm University, Faculty of Science, Department of Physics. Lund University, Sweden.
Stockholm University, Faculty of Science, Department of Physics.ORCID iD: 0000-0003-3444-1317
Number of Authors: 42021 (English)In: Electronic Structure, E-ISSN 2516-1075, Vol. 3, no 1, article id 014002Article in journal (Refereed) Published
Abstract [en]

A relativistic transient absorption theory is derived, implemented and validated within the dipole approximation based on the time-dependent Dirac equation. In the non-relativistic limit, it is found that the absorption agrees with the well established non-relativistic theory based on the time-dependent Schrodringer equation. Time-dependent simulations have been performed using the Dirac equation and the Schrodinger equation for the hydrogen atom in two different attosecond transient absorption scenarios. These simulations validate the present relativistic theory. The presented work can be seen as a first step in the development of a more general relativistic attosecond transient absorption spectroscopy method for studying heavy atoms, but it also suggests the possibility of studying relativistic effects, such as Zitterbewegung, in the time domain.

Place, publisher, year, edition, pages
2021. Vol. 3, no 1, article id 014002
Keywords [en]
Attosecond transient absorption, time dependent Dirac equation, relativistic velocity, gauge transformation, Zitterbewegung, power in quantum mechanics
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:su:diva-194542DOI: 10.1088/2516-1075/abe191ISI: 000645004100003Scopus ID: 2-s2.0-85106955050OAI: oai:DiVA.org:su-194542DiVA, id: diva2:1582678
Note

For corrigendum, see: Felipe Zapata et al 2022 Electron. Struct. 4 029501 DOI: 10.1088/2516-1075/ac646f

Available from: 2021-08-03 Created: 2021-08-03 Last updated: 2022-09-30Bibliographically approved

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Vinbladh, JimmyLindroth, Eva

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