Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Autoionizing Polaritons in Attosecond Atomic Ionization
Stockholm University, Faculty of Science, Department of Physics.ORCID iD: 0000-0003-3444-1317
Show others and affiliations
Number of Authors: 52021 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 127, no 2, article id 023202Article in journal (Refereed) Published
Abstract [en]

Light-induced states and Autler-Townes splitting of laser-coupled states are common features in the photoionization spectra of laser-dressed atoms. The entangled light-matter character of metastable Autler-Townes multiplets, which makes them autoionizing polaritons, however, is still largely unexplored. We employ attosecond transient-absorption spectroscopy in argon to study the formation of polariton multiplets between the 3s−14p and several light-induced states. We measure a controllable stabilization of the polaritons against ionization, in excellent agreement with ab initio theory. Using an extension of the Jaynes-Cummings model to autoionizing states, we show that this stabilization is due to the destructive interference between the Auger decay and the radiative ionization of the polaritonic components. These results give new insights into the optical control of electronic structure in the continuum and unlock the door to applications of radiative stabilization in metastable polyelectronic systems.

Place, publisher, year, edition, pages
2021. Vol. 127, no 2, article id 023202
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:su:diva-196009DOI: 10.1103/PhysRevLett.127.023202ISI: 000671590700006PubMedID: 34296926Scopus ID: 2-s2.0-85110079186OAI: oai:DiVA.org:su-196009DiVA, id: diva2:1589120
Available from: 2021-08-30 Created: 2021-08-30 Last updated: 2022-11-10Bibliographically approved

Open Access in DiVA

No full text in DiVA

Other links

Publisher's full textPubMedScopusarXiv:2103.17077

Authority records

Lindroth, Eva

Search in DiVA

By author/editor
Lindroth, Eva
By organisation
Department of Physics
In the same journal
Physical Review Letters
Physical Sciences

Search outside of DiVA

GoogleGoogle Scholar

doi
pubmed
urn-nbn

Altmetric score

doi
pubmed
urn-nbn
Total: 53 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf