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Switching of the electron-phonon interaction in 1T-VSe2 assisted by hot carriers
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Number of Authors: 232021 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 103, no 24, article id L241108Article in journal (Refereed) Published
Abstract [en]

We apply an intense infrared laser pulse in order to perturb the electronic and vibrational states in the three-dimensional charge density wave material 1T-VSe 2. Ultrafast snapshots of the light-induced hot carrier dynamics and nonequilibrium quasiparticle spectral function are collected using time- and angle-resolved photoemission spectroscopy. The hot carrier temperature and time-dependent electronic self-energy are extracted from the time-dependent spectral function, revealing that incoherent electron-phonon interactions heat the lattice above the charge density wave critical temperature on a timescale of (200 +/- 40) fs. Density functional perturbation theory calculations establish that the presence of hot carriers alters the overall phonon dispersion and quenches efficient low-energy acoustic phonon scattering channels, which results in a new quasiequilibrium state that is experimentally observed.

Place, publisher, year, edition, pages
2021. Vol. 103, no 24, article id L241108
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Materials Engineering Physical Sciences
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URN: urn:nbn:se:su:diva-195838DOI: 10.1103/PhysRevB.103.L241108ISI: 000662305100005OAI: oai:DiVA.org:su-195838DiVA, id: diva2:1589503
Available from: 2021-08-31 Created: 2021-08-31 Last updated: 2022-02-25Bibliographically approved

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Pakdel, SaharMarković, IgorLanatà, Nicola

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Nordic Institute for Theoretical Physics (Nordita)
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