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Peritectic Formation and Phase Stability of the Icosahedral Quasicystal i-GdCd and Its Ternary Variants with Zn, Mg, and Y
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
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Number of Authors: 52021 (English)In: Crystal Growth & Design, ISSN 1528-7483, E-ISSN 1528-7505, Vol. 21, no 6, p. 3355-3363Article in journal (Refereed) Published
Abstract [en]

Stable binary icosahedral quasicrystals (i-QCs) based on rare earth (RE) and cadmium are typically accessed by solution growth experiments, which operate in very narrow composition and temperature windows. Here, we present a procedure which allows study of peritectic reactions between approximant crystal (AC) phase and liquid yielding i-RECd and exemplify with i-GdCd and ternary variants where Cd is partially replaced by isovalent Zn (i-Gd(Cd,Zn)) or Mg (i-Gd(Cd,Mg)), or the 4f element Gd is replaced by nonmagnetic Y (i-(Gd,Y)Cd). The solubility limits for Zn and Mg substitution are about 10% and 20%, respectively, whereas Gd and Y show a complete solid solution behavior. We find that the peritectic decomposition temperature for i-GdCd is 390 degrees C, which is decreased when Gd is replaced by Y (i-YCd: 350 degrees C) and increased when Cd is replaced by Zn (i-Gd(Cd90Zn10): 440 degrees C), and especially by Mg (i-Gd(Cd80Mg20): 520 degrees C). Whereas substitution decisively alters the decomposition temperature (and hence stability) of the considered i-QCs, the decomposition temperature of the corresponding AC phases remains at around 700 degrees C. During the investigation of the pseudobinary phase diagrams Gd-(Cd95Zn5), Gd-(Cd90Zn10), and Gd-(Cd(80M)g(20)), faceted i-QCs grains with sizes up to 4 x 4 x 4 mm(3) could be isolated.

Place, publisher, year, edition, pages
2021. Vol. 21, no 6, p. 3355-3363
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Chemical Sciences Materials Engineering
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URN: urn:nbn:se:su:diva-196138DOI: 10.1021/acs.cgd.1c00147ISI: 000659409000023OAI: oai:DiVA.org:su-196138DiVA, id: diva2:1590365
Available from: 2021-09-02 Created: 2021-09-02 Last updated: 2022-03-23Bibliographically approved

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Eklöf, DanielGordeeva, AlisaHäussermann, Ulrich

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