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Light-induced shear phonon splitting and instability in bilayer graphene
Stockholm University, Nordic Institute for Theoretical Physics (Nordita). University of Bath, United Kingdom.ORCID iD: 0000-0002-9521-1008
Number of Authors: 12023 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 107, no 16, article id 165418Article in journal (Refereed) Published
Abstract [en]

Coherent engineering of landscape potential in crystalline materials is a rapidly evolving research field. Ultrafast optical pulses can manipulate low-frequency shear phonons in van der Waals layered materials through the dynamical dressing of electronic structure and photoexcited carrier density. In this work, we provide a diagrammatic formalism for nonlinear Raman force and implement it to shear phonon dynamics in bilayer graphene. We predict a controllable splitting of double degenerate shear phonon modes due to light-induced phonon mixing and renormalization according to a coherent nonlinear Raman force mechanism. Intriguingly, we obtain a light-induced shear phonon softening that facilitates structural instability at a critical field amplitude for which the shear phonon frequency vanishes. The phonon splitting and instability strongly depend on the laser intensity, frequency, chemical potential, and temperature of photoexcited electrons. This study motivates future experimental investigation of the optical fine tuning and regulation of shear phonons and layer stacking order in layered van der Waals materials.

Place, publisher, year, edition, pages
2023. Vol. 107, no 16, article id 165418
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:su:diva-218035DOI: 10.1103/PhysRevB.107.165418ISI: 000981079800004Scopus ID: 2-s2.0-85158830474OAI: oai:DiVA.org:su-218035DiVA, id: diva2:1784309
Available from: 2023-07-26 Created: 2023-07-26 Last updated: 2023-07-26Bibliographically approved

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Rostami, Habib

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