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Immobilization of Radionuclides on Iron Canister Material at Simulated Near-field Conditions
Stockholm University, Faculty of Science, Department of Environmental Chemistry.
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2009 (English)In: Scientific basis for nuclear waste management XXXII / [ed] Neil C. Hyatt, David A. Pickett, Raul B. Rebak, Warrendale, Pa: Materials Research Society , 2009, Vol. 1124, 111-116 p.Conference paper, Published paper (Refereed)
Abstract [en]

This work is a continuation of a long-term spent fuel leaching and radionuclides immobilization (by iron canister) experiment under simulated near-field conditions, in deoxygenated 2 mM NaHCO3 solution with 1 Gy/h g irradiation. The corrosion of iron canister material was investigated by electrochemical and microanalytical methods. Significant amounts of radionuclides (U, Np, Tc, Sr) were found to be immobilized on the corrosion layer of iron canister material by using SEM_WDS and SIMS methods. The observation is useful for bettering our understanding of near-field chemical processes at earlier canister failure conditions.

Place, publisher, year, edition, pages
Warrendale, Pa: Materials Research Society , 2009. Vol. 1124, 111-116 p.
Series
Materials Research Society symposia proceedings, ISSN 0272-9172 ; 1124
National Category
Environmental Sciences
Research subject
Environmental Chemistry
Identifiers
URN: urn:nbn:se:su:diva-34396OAI: oai:DiVA.org:su-34396DiVA: diva2:289007
Conference
Materials Research Society. Fall Meeting 2008, Boston. Symposium Q
Available from: 2010-01-22 Created: 2010-01-08 Last updated: 2011-05-17Bibliographically approved

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