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Control of Electron Localization in Deuterium Molecular Ions using an Attosecond Pulse Train and a Many-Cycle Infrared Pulse
Stockholm University, Faculty of Science, Department of Physics.
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2010 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 104, no 2, 23001- p.Article in journal (Refereed) Published
Abstract [en]

We demonstrate an experimental control of electron localization in deuterium molecular ions created and dissociated by the combined action of an attosecond pulse train and a many-cycle infrared (IR) pulse. The attosecond pulse train is synthesized using both even and odd high order harmonics of the driving IR frequency so that it can strobe the IR field once per IR cycle. An asymmetric ejection of the deuterium ions oscillates with the full IR period when the APT-IR time-delay is scanned. The observed control is due to the creation of a coherent superposition of 1s sigma(g) and 2p sigma(u) states via interference between one-photon and two-photon dissociation channels.

Place, publisher, year, edition, pages
2010. Vol. 104, no 2, 23001- p.
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Natural Sciences
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URN: urn:nbn:se:su:diva-49693DOI: 10.1103/PhysRevLett.104.023001ISI: 000274002900017OAI: oai:DiVA.org:su-49693DiVA: diva2:379340
Note
authorCount :13Available from: 2010-12-17 Created: 2010-12-17 Last updated: 2017-12-11Bibliographically approved

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