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Magic and hot giant fullerenes formed inside ion irradiated weakly bound C-60 clusters
Stockholm University, Faculty of Science, Department of Physics.
Stockholm University, Faculty of Science, Department of Physics.
Stockholm University, Faculty of Science, Department of Physics.
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2010 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 133, no 10, 104301- p.Article in journal (Refereed) Published
Abstract [en]

We find that the most stable fullerene isomers, C-70-C-94, form efficiently in close-to central collisions between keV atomic ions and weakly bound clusters of more than 15 C-60-molecules. We observe extraordinarily high yields of C-70 and marked preferences for C-78 and C-84. Larger even-size carbon molecules, C-96-C-180, follow a smooth log-normal (statistical) intensity distribution. Measurements of kinetic energies indicate that C-70-C-94 mainly are formed by coalescence reactions between small carbon molecules and Coo, while C-n with n >= 96 are due to self-assembly (of small molecules) and shrinking hot giant fullerenes.

Place, publisher, year, edition, pages
2010. Vol. 133, no 10, 104301- p.
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Natural Sciences
Identifiers
URN: urn:nbn:se:su:diva-51757DOI: 10.1063/1.3479584ISI: 000282475400015OAI: oai:DiVA.org:su-51757DiVA: diva2:386001
Note
authorCount :13Available from: 2011-01-12 Created: 2011-01-12 Last updated: 2017-12-11Bibliographically approved

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