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Highly enantioselective co-catalytic direct aldol reactions by combination of hydrogen-bond donating and acyclic amino acid catalysts
Mid Sweden University, Department of Natural Sciences, Engineering and Mathematics.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Mid Sweden University, Department of Natural Sciences, Engineering and Mathematics.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
2011 (English)In: Advanced Synthesis and Catalysis, ISSN 1615-4150, E-ISSN 1615-4169, Vol. 353, no 17, 3114-3122 p.Article in journal (Refereed) Published
Abstract [en]

Highly enantioselective co-catalytic direct aldol reactions by a combination of simple hydrophobic acyclic amino acid and hydrogen-bond donating catalysts are presented. The corresponding aldol products are formed in high yields with high regio-, diastereo- (anti or syn) and enantioselectivity (up to 99.5:0.5 er). The catalyst loadings can be decreased to as little as 2 mol%.

Place, publisher, year, edition, pages
Wiley-VCH Verlagsgesellschaft, 2011. Vol. 353, no 17, 3114-3122 p.
Keyword [en]
aldol reaction, amino acids, asymmetric catalysis, co-catalysis, hydrogen-bond donating
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-65524DOI: 10.1002/adsc.201100408ISI: 000298171500007OAI: oai:DiVA.org:su-65524DiVA: diva2:464020
Funder
Swedish Research Council
Available from: 2011-12-12 Created: 2011-12-12 Last updated: 2017-12-08Bibliographically approved

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