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Unique water-water coordination tailored by a metal surface
Stockholm University, Faculty of Science, Department of Physics. SLAC National Accelerator Laboratory .
Stockholm University, Faculty of Science, Department of Physics.
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2013 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 138, no 23, 234708- p.Article in journal (Refereed) Published
Abstract [en]

At low coverage of water on Cu(110), substrate-mediated electrostatics lead to zigzagging chains along [001] as observed with STM [T. Yamada, S. Tamamori, H. Okuyama, and T. Aruga, Anisotropic water chain growth on Cu(110) observed with scanning tunneling microscopy Phys. Rev. Lett. 96, 036105 (2006)]. Using x-ray absorption spectroscopy we find an anomalous low-energy resonance at similar to 533.1 eV which, based on density functional theory spectrum simulations, we assign to an unexpected configuration of water units whose uncoordinated O-H bonds directly face those of their neighbors; this interaction repeats over trough sites with enhanced electron density and is analogous to the case of a hydrated electron.

Place, publisher, year, edition, pages
2013. Vol. 138, no 23, 234708- p.
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Physical Sciences
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URN: urn:nbn:se:su:diva-92654DOI: 10.1063/1.4809680ISI: 000321012400033OAI: oai:DiVA.org:su-92654DiVA: diva2:640857
Note

AuthorCount:10;

Available from: 2013-08-14 Created: 2013-08-14 Last updated: 2017-12-06Bibliographically approved

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