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Palladium-Catalyzed Oxidative Carbocyclization-Carbonylation of Allenynes and Enallenes
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
2014 (English)In: Chemistry - A European Journal, ISSN 0947-6539, E-ISSN 1521-3765, Vol. 20, no 25, 7608-7612 p.Article in journal (Refereed) Published
Abstract [en]

A highly efficient oxidative carbocyclization-carbonylation reaction cascade of allenynes and enallenes has been developed using a Pd-II salt in low catalytic amounts under ambient temperature and pressure (1 atm of carbon monoxide). The use of DMSO as an additive was found to be important for an efficient reaction. A wide range of alcohols as trapping reagents were used to give the corresponding esters in good yields.

Place, publisher, year, edition, pages
Weinheim: Wiley-VCH Verlag GmbH & Co. KGaA , 2014. Vol. 20, no 25, 7608-7612 p.
Keyword [en]
carbocyclization, carbonylation, homogeneous catalysis, oxidation, palladium
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-106295DOI: 10.1002/chem.201402688ISI: 000337637400011OAI: oai:DiVA.org:su-106295DiVA: diva2:735848
Funder
EU, European Research Council, ERC AdG 247014Swedish Research CouncilWenner-Gren Foundations
Note

AuthorCount:3;

Available from: 2014-08-01 Created: 2014-08-01 Last updated: 2017-12-05Bibliographically approved

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Volla, Chandra M. R.Mazuela, JavierBäckvall, Jan-Erling
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