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Spectroscopy and picosecond dynamics of aqueous NO2
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2014 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 141, no 6, 064310- p.Article in journal (Refereed) Published
Abstract [en]

We investigate the formation of aqueous nitrogen dioxide, NO2 formed through femtosecond photolysis of nitrate, NO3- ( aq) and nitromethane CH3NO2(aq). Common to the experiments is the observation of a strong induced absorption at 1610 +/- 10 cm(-1), assigned to the asymmetric stretch vibration in the ground state of NO2. This assignment is substantiated through isotope experiments substituting N-14 by N-15, experiments at different pH values, and by theoretical calculations and simulations of NO2-D2O clusters.

Place, publisher, year, edition, pages
2014. Vol. 141, no 6, 064310- p.
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Physical Sciences
URN: urn:nbn:se:su:diva-107623DOI: 10.1063/1.4892342ISI: 000340713700032OAI: diva2:749752


Available from: 2014-09-25 Created: 2014-09-22 Last updated: 2014-09-25Bibliographically approved

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Jena, Naresh K.Odelius, Michael
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Department of Physics
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