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A 3D 12-Ring Zeolite with Ordered 4-Ring Vacancies Occupied by (H2O)(2) Dimers
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK). Peking University, People's Republic of China.
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
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2014 (English)In: Chemistry - A European Journal, ISSN 0947-6539, E-ISSN 1521-3765, Vol. 20, no 49, 16097-16101 p.Article in journal (Refereed) Published
Abstract [en]

A germanate zeolite, PKU-14, with a three- dimensional large-pore channel system was structurally characterized by a combination of high-resolution powder X-ray diffraction, rotation electron diffraction, NMR, and IR spectroscopy. Ordered Ge4O4 vacancies inside the [4(6).6(12)] cages has been found in PKU-14, in which a unique (H2O)(2) dimer was located at the vacancies and played a structure-directing role. It is the first time that water clusters are found to be templates for ordered framework vacancies.

Place, publisher, year, edition, pages
2014. Vol. 20, no 49, 16097-16101 p.
Keyword [en]
electron microscopy, porous materials, structure elucidation, zeolite analogues, X-ray diffraction
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:su:diva-111418DOI: 10.1002/chem.201405449ISI: 000345515700011OAI: oai:DiVA.org:su-111418DiVA: diva2:775746
Note

AuthorCount:8;

Available from: 2015-01-05 Created: 2015-01-02 Last updated: 2017-12-05Bibliographically approved

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Liang, JieSu, JieZou, XiaodongSun, Junliang
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