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Preparation of Tetrasubstituted Olefins Using Mono or Double Aerobic Direct C-H Functionalization Strategies: Importance of Steric Effects
Stockholm University, Faculty of Science, Department of Organic Chemistry. Université Paris-Sud, France.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
2015 (English)In: Journal of Organic Chemistry, ISSN 0022-3263, E-ISSN 1520-6904, Vol. 80, no 5, 2796-2803 p.Article in journal (Refereed) Published
Abstract [en]

A novel protocol for the synthesis of tetrasubstituted olefins through a biomimetic approach has been explored. Both mono- and diarylations were performed under ambient oxygen pressure, giving a range of highly hindered tetrasubstituted alkenes. For diarylation of disubstituted substrates, it was demonstrated that the second arylation is the rate-limiting step of the overall transformation.

Place, publisher, year, edition, pages
2015. Vol. 80, no 5, 2796-2803 p.
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-116625DOI: 10.1021/acs.joc.5b00148ISI: 000350841600033PubMedID: 25653084OAI: oai:DiVA.org:su-116625DiVA: diva2:808190
Funder
EU, European Research CouncilSwedish Research CouncilKnut and Alice Wallenberg Foundation
Note

AuthorCount:3;

Available from: 2015-04-27 Created: 2015-04-22 Last updated: 2017-12-04Bibliographically approved

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