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Effect of the functionalisation route on a Zr-MOF with an Ir-NHC complex for catalysis
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
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2015 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 51, no 54, 10864-10867 p.Article in journal (Refereed) Published
Abstract [en]

A new iridium N-heterocyclic carbene (NHC) metallolinker has been synthesised and introduced into a metal-organic framework (MOF), for the first time, via two different routes: direct synthesis and postsynthetic exchange (PSE). The two materials were compared in terms of the Ir loading and distribution using X-ray energy dispersive spectroscopy (EDS), the local Ir structure using X-ray absorption spectroscopy (XAS) and the catalytic activity. The materials showed good activity and recyclability as catalysts for the isomerisation of an allylic alcohol.

Place, publisher, year, edition, pages
2015. Vol. 51, no 54, 10864-10867 p.
National Category
Organic Chemistry
Research subject
Organic Chemistry
Identifiers
URN: urn:nbn:se:su:diva-119026DOI: 10.1039/c5cc03934gISI: 000356717000018OAI: oai:DiVA.org:su-119026DiVA: diva2:843053
Funder
Swedish Research CouncilVINNOVAKnut and Alice Wallenberg Foundation
Available from: 2015-07-24 Created: 2015-07-24 Last updated: 2017-11-07Bibliographically approved

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Carson, FabianMartínez-Castro, ElisaMarcos, RocioGonzález Miera, GrecoJansson, KjellZou, XiaodongMartin-Matute, Belén
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