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A decline in Arctic Ocean mercury suggested by differences in decadal trends of atmospheric mercury between the Arctic and northern midlatitudes
Stockholm University, Faculty of Science, Department of Environmental Science and Analytical Chemistry. Harvard University, USA.
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Number of Authors: 8
2015 (English)In: Geophysical Research Letters, ISSN 0094-8276, E-ISSN 1944-8007, Vol. 42, no 14, 6076-6083 p.Article in journal (Refereed) Published
Abstract [en]

Atmospheric mercury (Hg) in the Arctic shows much weaker or insignificant annual declines relative to northern midlatitudes over the past decade (2000-2009) but with strong seasonality in trends. We use a global ocean-atmosphere model of Hg (GEOS-Chem) to simulate these observed trends and determine the driving environmental variables. The atmospheric decline at northern midlatitudes can largely be explained by decreasing North Atlantic oceanic evasion. The midlatitude atmospheric signal propagates to the Arctic but is countered by rapid Arctic warming and declining sea ice, which suppresses deposition and promotes oceanic evasion over the Arctic Ocean. The resulting simulation implies a decline of Hg in the Arctic surface ocean that we estimate to be -0.67%yr(-1) over the study period. Rapid Arctic warming and declining sea ice are projected for future decades and would drive a sustained decline in Arctic Ocean Hg, potentially alleviating the methylmercury exposure risk for northern populations.

Place, publisher, year, edition, pages
2015. Vol. 42, no 14, 6076-6083 p.
Keyword [en]
mercury, Arctic, trend, climatological variables
National Category
Earth and Related Environmental Sciences
Identifiers
URN: urn:nbn:se:su:diva-120706DOI: 10.1002/2015GL064051ISI: 000359316100049OAI: oai:DiVA.org:su-120706DiVA: diva2:854753
Available from: 2015-09-17 Created: 2015-09-15 Last updated: 2017-12-04Bibliographically approved

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Sörensen, Anne L.
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