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Majchrzak, P., Pakdel, S., Biswas, D., Jones, A. J. H., Volckaert, K., Marković, I., . . . Ulstrup, S. (2021). Switching of the electron-phonon interaction in 1T-VSe2 assisted by hot carriers. Physical Review B, 103(24), Article ID L241108.
Open this publication in new window or tab >>Switching of the electron-phonon interaction in 1T-VSe2 assisted by hot carriers
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2021 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 103, no 24, article id L241108Article in journal (Refereed) Published
Abstract [en]

We apply an intense infrared laser pulse in order to perturb the electronic and vibrational states in the three-dimensional charge density wave material 1T-VSe 2. Ultrafast snapshots of the light-induced hot carrier dynamics and nonequilibrium quasiparticle spectral function are collected using time- and angle-resolved photoemission spectroscopy. The hot carrier temperature and time-dependent electronic self-energy are extracted from the time-dependent spectral function, revealing that incoherent electron-phonon interactions heat the lattice above the charge density wave critical temperature on a timescale of (200 +/- 40) fs. Density functional perturbation theory calculations establish that the presence of hot carriers alters the overall phonon dispersion and quenches efficient low-energy acoustic phonon scattering channels, which results in a new quasiequilibrium state that is experimentally observed.

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Materials Engineering Physical Sciences
Identifiers
urn:nbn:se:su:diva-195838 (URN)10.1103/PhysRevB.103.L241108 (DOI)000662305100005 ()
Available from: 2021-08-31 Created: 2021-08-31 Last updated: 2022-02-25Bibliographically approved
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ORCID iD: ORCID iD iconorcid.org/0000-0002-1631-9556

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