A search for the Higgs boson decaying into a photon and a pair of electrons or muons with an invariant mass m(ll) < 30 GeV is presented. The analysis is performed using 139 fb(-1) of proton-proton collision data, produced by the LHC at a centre-of-mass energy of 13 TeV and collected by the ATLAS experiment. Evidence for the H -> ll(gamma) process is found with a significance of 3.2 over the background-only hypothesis, compared to an expected significance of 2.1 for the Standard Model prediction. The best-fit value of the signal-strength parameter, defined as the ratio of the observed signal yield to the one expected in the Standard Model, is mu = 1.5 +/- 0.5. The Higgs boson production cross-section times the H -> ll(gamma) branching ratio for m(ll) < 30 GeV is determined to be 8.7(-2.7)(+2.8) fb.