Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Relativistic Two-Photon Matrix Elements for Attosecond Delays
Stockholm University, Faculty of Science, Department of Physics.
Stockholm University, Faculty of Science, Department of Physics.ORCID iD: 0000-0003-3444-1317
Number of Authors: 32022 (English)In: Atoms, E-ISSN 2218-2004, Vol. 10, no 3, article id 80Article in journal (Refereed) Published
Abstract [en]

The theory of one-photon ionization and two-photon above-threshold ionization is formulated for applications to heavy atoms in attosecond science by using Dirac–Fock formalism. A direct comparison of Wigner–Smith–Eisenbud delays for photoionization is made with delays from the Reconstruction of Attosecond Beating By Interference of Two-photon Transitions (RABBIT) method. Photoionization by an attosecond pulse train, consisting of monochromatic fields in the extreme ultraviolet range, is computed with many-body effects at the level of the relativistic random phase approximation (RRPA). Subsequent absorption and emission processes of infrared laser photons in RABBIT are evaluated by using static ionic potentials as well as asymptotic properties of relativistic Coulomb functions. As expected, light elements, such as argon, show negligible relativistic effects, whereas heavier elements, such a krypton and xenon, exhibit delays that depend on the fine-structure of the ionic target. The relativistic effects are notably close to ionization thresholds and Cooper minima with differences in fine-structure delays predicted to be as large as tens of attoseconds. The separability of relativistic RABBIT delays into a Wigner–Smith–Eisenbud delay and a universal continuum–continuum delay is studied with reasonable separability found for photoelectrons emitted along the laser polarization axis in agreement with prior non-relativistic results.

Place, publisher, year, edition, pages
2022. Vol. 10, no 3, article id 80
Keywords [en]
attoscience, attophysics, photoionization, above-threshold ionization, Wigner-Smith-Eisenbud delay, Dirac-Fock, RRPA, RABBIT, krypton, xenon
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:su:diva-210274DOI: 10.3390/atoms10030080ISI: 000857381700001Scopus ID: 2-s2.0-85138713905OAI: oai:DiVA.org:su-210274DiVA, id: diva2:1702939
Available from: 2022-10-12 Created: 2022-10-12 Last updated: 2022-10-12Bibliographically approved

Open Access in DiVA

No full text in DiVA

Other links

Publisher's full textScopus

Authority records

Vinbladh, JimmyLindroth, Eva

Search in DiVA

By author/editor
Vinbladh, JimmyLindroth, Eva
By organisation
Department of Physics
In the same journal
Atoms
Atom and Molecular Physics and Optics

Search outside of DiVA

GoogleGoogle Scholar

doi
urn-nbn

Altmetric score

doi
urn-nbn
Total: 81 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf