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Isotopic apportionment of sulfate aerosols between natural and anthropogenic sources in the outflow of South Asia
Stockholm University, Faculty of Science, Department of Environmental Science.
Stockholm University, Faculty of Science, Department of Environmental Science. Stockholm University, Faculty of Science, The Bolin Centre for Climate Research (together with KTH & SMHI).ORCID iD: 0000-0002-5724-8256
Stockholm University, Faculty of Science, Department of Environmental Science. Stockholm University, Faculty of Science, The Bolin Centre for Climate Research (together with KTH & SMHI).
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Number of Authors: 82026 (English)In: Atmospheric Chemistry And Physics, ISSN 1680-7316, E-ISSN 1680-7324, Vol. 26, no 8, p. 5333-5343Article in journal (Refereed) Published
Abstract [en]

Sulfate aerosols cool the climate and thus temporarily mask climate warming, but at a cost to air quality. Their short atmospheric lifetime leads to heterogeneous global coverage, with sulfate concentrations over South Asia being especially elevated and continuing to increase. It remains challenging to constrain the relative importance of different emission sources due to poor observational coverage and uncertainties in bottom-up technology-based emission estimates. The stable sulfur isotope composition (delta 34S-SO42-) quantitatively distinguishes natural and anthropogenic sources. This study aimed to constrain the sources of sulfate arriving at the Maldives Climate Observatory Hanimaadhoo (MCOH), which is ideally situated for intercepting the outflow from airsheds over the Indian subcontinent. The results show that anthropogenic sources of sulfate contributed 93 +/- 14 %, 87 +/- 10 %, and 66 +/- 12 % in winter (post-monsoon), spring (pre-monsoon), and summer (monsoon), respectively. There was also a moderate to strong correlation (r2= 0.75, p << 0.05, n=7) between continental anthropogenic (winter and spring) sulfate (delta 34S) and black carbon aerosols from fossil fuel combustion (pinpointed by Delta 14C). This study provides improved constraints on sulfate sources for South Asia - a key region for aerosol pollution and aerosol masking of climate warming.

Place, publisher, year, edition, pages
2026. Vol. 26, no 8, p. 5333-5343
National Category
Meteorology and Atmospheric Sciences
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URN: urn:nbn:se:su:diva-255523DOI: 10.5194/acp-26-5333-2026ISI: 001744785800001Scopus ID: 2-s2.0-105036637193OAI: oai:DiVA.org:su-255523DiVA, id: diva2:2060582
Available from: 2026-05-18 Created: 2026-05-18 Last updated: 2026-05-18Bibliographically approved

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Holmstrand, HenryRemani, ManojHaslett, SophieGustafsson, Örjan

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