Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Electron spin resonance and ferromagnetic resonance spectroscopy in the high-field phase of the van der Waals magnet CrCl3
Stockholm University, Faculty of Science, Department of Materials and Environmental Chemistry (MMK).
Show others and affiliations
Number of Authors: 82020 (English)In: Physical Review Materials, E-ISSN 2475-9953, Vol. 4, no 6, article id 064406Article in journal (Refereed) Published
Abstract [en]

We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl3. This material, although being known for quite a while, has received recent significant attention in a context of the use of van der Waals magnets in novel spintronic devices. Temperature-dependent measurements of the resonance fields were performed between 4 and 175 K and with the external magnetic field applied parallel and perpendicular to the honeycomb planes of the crystal structure. These investigations reveal that the resonance line shifts from the paramagnetic resonance position already at temperatures well above the transition into a magnetically ordered state. Thereby the existence of ferromagnetic short-range correlations above the transition is established and the intrinsically two-dimensional nature of the magnetism in the title compound is proven. To study details of the magnetic anisotropies in the field-induced effectively ferromagnetic state at low temperatures, frequency-dependent ferromagnetic resonance (FMR) measurements were conducted at 4 K. The observed anisotropy between the two magnetic-field orientations is analyzed by means of numerical simulations based on a phenomenological theory of FMR. These simulations are in excellent agreement with measured data if the shape anisotropy of the studied crystal is taken into account, while the magnetocrystalline anisotropy is found to be negligible in CrCl3. The absence of a significant intrinsic anisotropy thus renders this material as a practically ideal isotropic Heisenberg magnet.

Place, publisher, year, edition, pages
2020. Vol. 4, no 6, article id 064406
Keywords [en]
Magnetic anisotropy
National Category
Materials Engineering
Identifiers
URN: urn:nbn:se:su:diva-182842DOI: 10.1103/PhysRevMaterials.4.064406ISI: 000537621500002OAI: oai:DiVA.org:su-182842DiVA, id: diva2:1458549
Available from: 2020-08-17 Created: 2020-08-17 Last updated: 2022-02-26Bibliographically approved

Open Access in DiVA

No full text in DiVA

Other links

Publisher's full text

Authority records

Roslova, Maria

Search in DiVA

By author/editor
Roslova, Maria
By organisation
Department of Materials and Environmental Chemistry (MMK)
In the same journal
Physical Review Materials
Materials Engineering

Search outside of DiVA

GoogleGoogle Scholar

doi
urn-nbn

Altmetric score

doi
urn-nbn
Total: 118 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf